单光子和双光子吸收 原理和应用PDF电子书下载

CHAPTER 1 One-Photon Absorption Theory 1

References 3

CHAPTER 2 Charge Transfer and Electron-Hole Coherence in OPA 5

References 7

CHAPTER 3 Application of OPA 9

3.1 Biology 9

3.1.1 Retinal proteins（rhodopsins） 9

3.1.2 Green fluorescent protein 16

3.2 Enenrgy materials 24

3.2.1 Quinoidal charge delocalization in poly-p-phenylene cation radical 24

3.2.2 Neutral and charged π-dimeric quinquethiophenes 31

3.2.3 Surface-enhanced resonance Raman scattering 39

3.2.4 Near- and deep-UV resonance Raman spectroscopy of pyrazine-Al4 complex and Al3-pyrazine-Al3 junction 51

References 60

CHAPTER 4 Two-Photon Absorption 71

4.1 TPA section 71

4.2 Experimental methods and TPA materials 74

References 80

CHAPTER 5 Polarizabilities in Absorption Processes 83

References 85

CHAPTER 6 Charge Transfer and Electron-Hole Coherence in TPA 86

6.1 3D cube and 2D site representations for TPA 86

6.2 Quantum chemical calculations 88

6.3 Visualizations of transition dipoles,charge transfer and electron-hole coherence on electronic state transitions between excited states for TPA 91

6.4 Photoexcitation mechanisms of centrosymmetric and asymmetric fluorine derivatives in TPA 98

References 110

CHAPTER 7 Application of TPA 113

7.1 Two-photon photophysical properties of tri-9-anthrylborane 113

7.2 Spectroscopic and theoretical studies on the photophysical properties of dichlorotriazine derivatives 124

References 133

CHAPTER 8 Modeling Examples of Photon Absorptions and Nonlinear Properties in Pro-Aromatic Chromophores 138

References 150

CHAPTER 9 Modeling Examples of Simulated Polymethine Dyes for All-Optical Witching 154

Summary 165

References 165

Acknowledgements 168